Priscila Rosa, Yuanfeng Xu, Marein Rahn, Jean Souza, Satya Kushwaha, Larissa Veiga, Alessandro Bombardi, Sean Thomas, Marc Janoschek, Eric Bauer, Mun Chan, Zhijun Wang, Joe Thompson, Neil Harrison, Pascoal Pagliuso, Andrei Bernevig, Filip Ronning
- Here we investigate antiferromagnetic Eu5In2Sb6, a nonsymmorphic Zintl phase. Our electrical transport data show that Eu5In2Sb6 is remarkably insulating and exhibits an exceptionally large negative magnetoresistance, which is consistent with the presence of magnetic polarons. From ab initio calculations, the paramagnetic state of Eu5In2Sb6 is a topologically nontrivial semimetal within the generalized gradient approximation (GGA), whereas an insulating state with trivial topological indices is obtained using a modified Becke−Johnson potential. Notably, GGA + U calculations suggest that the antiferromagnetic phase of Eu5In2Sb6 may host an axion insulating state. Our results provide important feedback for theories of topological classification and highlight the potential of realizing clean magnetic narrow-gap semiconductors in Zintl materials.
