All-optical magnetization switching of GdFe by double-pulse laser excitation

  • The tremendous interest in the technology and underlying physics of all-optical switching of magnetization brings up the question of how fast the switching can occur and how high the frequency of writing the data with ultrafast laser pulses can be. To answer this question, we excited a GdFe ferrimagnetic alloy, the magnetization of which can be reversed by single laser pulses, a phenomenon known as toggle switching, by two pulses with a certain time delay in between. Using photoemission electron microscopy and Kerr microscopy for magnetic domain imaging, we explore the effects of varying fluences of the first and second pulse as well as the time delay between the two pulses. Our results show that when the fluence of the first pulse is adjusted just above the threshold of single-pulse switching, a second pulse with about 60 % of the fluence of the first pulse, arriving only 3 ps later, switches the magnetization back. This reswitching persists up to about 40 ps pulse separation. WeThe tremendous interest in the technology and underlying physics of all-optical switching of magnetization brings up the question of how fast the switching can occur and how high the frequency of writing the data with ultrafast laser pulses can be. To answer this question, we excited a GdFe ferrimagnetic alloy, the magnetization of which can be reversed by single laser pulses, a phenomenon known as toggle switching, by two pulses with a certain time delay in between. Using photoemission electron microscopy and Kerr microscopy for magnetic domain imaging, we explore the effects of varying fluences of the first and second pulse as well as the time delay between the two pulses. Our results show that when the fluence of the first pulse is adjusted just above the threshold of single-pulse switching, a second pulse with about 60 % of the fluence of the first pulse, arriving only 3 ps later, switches the magnetization back. This reswitching persists up to about 40 ps pulse separation. We interpret the latter as the time required for the sample to cool down and remagnetize after the first pulse. For shorter time delays below about 2 ps, no reswitching occurs. However, the effect of the two pulses adds up, enabling switching for fluences of both pulses below the threshold for single-pulse switching. Atomistic spin dynamics simulations are used to model the experimental data, successfully confirming our results.show moreshow less

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Author:Rahil Hosseinifar, Felix Steinbach, Ivar Kumberg, José Miguel Lendínez, Sangeeta Thakur, Sebastien E. Hadjadj, Jendrik Gördes, Chowdhury S. Awsaf, Mario Fix, Manfred AlbrechtORCiDGND, Florian Kronast, Unai Atxitia, Clemens von Korff Schmising, Wolfgang Kuch
URN:urn:nbn:de:bvb:384-opus4-1280775
Frontdoor URLhttps://opus.bibliothek.uni-augsburg.de/opus4/128077
ISSN:2469-9950OPAC
ISSN:2469-9969OPAC
Parent Title (English):Physical Review B
Publisher:American Physical Society (APS)
Place of publication:College Park, MD
Type:Article
Language:English
Year of first Publication:2025
Publishing Institution:Universität Augsburg
Release Date:2026/02/11
Volume:112
Issue:17
First Page:174406
DOI:https://doi.org/10.1103/h8j7-4f2z
Institutes:Mathematisch-Naturwissenschaftlich-Technische Fakultät
Mathematisch-Naturwissenschaftlich-Technische Fakultät / Institut für Physik
Mathematisch-Naturwissenschaftlich-Technische Fakultät / Institut für Physik / Lehrstuhl für Experimentalphysik V
Dewey Decimal Classification:5 Naturwissenschaften und Mathematik / 53 Physik / 530 Physik
Licence (German):CC-BY 4.0: Creative Commons: Namensnennung