Nonthermal electron-photon steady states in open cavity quantum materials

  • Coupling a system to two different baths can lead to novel phenomena escaping the constraints of thermal equilibrium. In quantum materials inside optical cavities, this feature can be exploited as electrons and cavity photons are easily pulled away from their mutual equilibrium, even in the steady state. This offers new routes for a noninvasive control of material properties and functionalities. We show that the absence of thermal equilibrium between electrons and photons leads to reduced symmetries of the steady-state electronic distribution function. Moreover, by defining an effective temperature from the on-shell distribution function, we find a nonmonotonic behavior as a function of cavity frequency, consistent with recent experimental findings. Finally, we show that, the nonthermal behavior leads to qualitative modifications of the materials properties, as the standard Sommerfeld expansion for observables is modified by a leading-order correction linearly proportional to theCoupling a system to two different baths can lead to novel phenomena escaping the constraints of thermal equilibrium. In quantum materials inside optical cavities, this feature can be exploited as electrons and cavity photons are easily pulled away from their mutual equilibrium, even in the steady state. This offers new routes for a noninvasive control of material properties and functionalities. We show that the absence of thermal equilibrium between electrons and photons leads to reduced symmetries of the steady-state electronic distribution function. Moreover, by defining an effective temperature from the on-shell distribution function, we find a nonmonotonic behavior as a function of cavity frequency, consistent with recent experimental findings. Finally, we show that, the nonthermal behavior leads to qualitative modifications of the materials properties, as the standard Sommerfeld expansion for observables is modified by a leading-order correction linearly proportional to the temperature difference between the two baths and to the frequency derivative of the electron damping.show moreshow less

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Metadaten
Author:R. Flores-Calderón, Md Mursalin Islam, Michele Pini, Francesco PiazzaORCiDGND
URN:urn:nbn:de:bvb:384-opus4-1217298
Frontdoor URLhttps://opus.bibliothek.uni-augsburg.de/opus4/121729
ISSN:2643-1564OPAC
Parent Title (English):Physical Review Research
Publisher:American Physical Society (APS)
Place of publication:College Park, MD
Type:Article
Language:English
Year of first Publication:2025
Publishing Institution:Universität Augsburg
Release Date:2025/05/05
Volume:7
Issue:1
First Page:013073
DOI:https://doi.org/10.1103/physrevresearch.7.013073
Institutes:Mathematisch-Naturwissenschaftlich-Technische Fakultät
Mathematisch-Naturwissenschaftlich-Technische Fakultät / Institut für Physik
Mathematisch-Naturwissenschaftlich-Technische Fakultät / Institut für Physik / Lehrstuhl für Theoretische Physik III
Dewey Decimal Classification:5 Naturwissenschaften und Mathematik / 53 Physik / 530 Physik
Licence (German):CC-BY 4.0: Creative Commons: Namensnennung (mit Print on Demand)